Fully Printed Flexible Smart Hybrid Hydrogels

Yang ZHOU, Michael LAYANI, Shancheng WANG, Peng HU, Yujie KE, Shlomo MAGDASSI*, Yi LONG

*Corresponding author for this work

Research output: Journal PublicationsJournal Article (refereed)peer-review

148 Citations (Scopus)

Abstract

A printable hybrid hydrogel is fabricated by embedding poly(N-isopropylacrylamide) (PNIPAm) microparticles within a water-rich silica-alumina(Si/Al)-based gel matrix. The hybrid gel holds water content of up to 70 wt%, due to its unique Si/Al matrix. The hybrid hydrogel can respond to both heat and electrical stimuli, and can be directly printed layer-by-layer using a commercial 3-dimensional printer, without requiring any curing. The hybrid ink is printed onto a transparent, flexible conductive electrode composed of silver nanoparticles and sustains bending angles of up to 180°, which enables patterning of various flexible devices such as smart windows and a 3D optical waveguide valve.
Original languageEnglish
Article number1705365
Number of pages8
JournalAdvanced Functional Materials
Volume28
Issue number9
Early online date8 Jan 2018
DOIs
Publication statusPublished - 28 Feb 2018
Externally publishedYes

Bibliographical note

Publisher Copyright:
© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

Funding

The work was supported by the National Research Foundation, the Prime Minister's Office, and Singapore, under its Campus for Research Excellence and Technological Enterprise (CREATE) program.

Keywords

  • 3D printing
  • hydrogels
  • PNIPAm
  • smart windows
  • thermochromics

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